Dear Harry,
we recently ran Black Shale samples (Toarcian) for isotopic C and N and
C/N ratios using the automated GC-MS Carlo
Erba-SymbolDS. Our samples ranged
from 0.1 to 10% for TOC and from 10 to 90% for Total Carbon.
We tried two different ways to isolate kerogen from our sediment:
HCl demineralization
HF-BF3 maceration (Robl et ali 1993-Org.Geochem. Vol 20, n°2,
pp249-255).
The HCl demineralized samples gave insufficient concentrated organic
matter for C/N and N isotopic analyses.
The HF-BF3 tecnique resulted in a final de-ashed product which is
sufficiently concentrated in OM for all of our purposes.
Elemental analysis of delta 13C-org did not indicate any significant
difference in organic alteration using the HCl or HF-BF3 technique.
good luck,
Antonio
Antonio Bacheca
Institute de Mineralogie et Petrographie
Université de Lausanne
BFSH-2 1015 Dorigny
Suisse