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this is a google news search for the exact term "21st century skills" earliest ref 
is 1990. But it obviously does not include all material...

http://news.google.com/archivesearch?q=%2221st+century+skills%
22&scoring=a&hl=en&ned=us&sa=N&sugg=d&as_ldate=1990&as_hdate=1991&ln
av=hist0

For another approach try and hitup the people at PFTCS, maybe they know.

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R.